A criterion for the freezing of a liquid is investigated through an analysis of the contribution of multiparticle correlations to the statistical entropy. Molecular-dynamics results are presented for a Lennard-Jones system at two subcritical isotherms in a range of densities across the freezing line.
ENTROPY AND THE FREEZING OF SIMPLE LIQUIDS
GIAQUINTA, Paolo Vittorio;PRESTIPINO GIARRITTA, Santi
1992-01-01
Abstract
A criterion for the freezing of a liquid is investigated through an analysis of the contribution of multiparticle correlations to the statistical entropy. Molecular-dynamics results are presented for a Lennard-Jones system at two subcritical isotherms in a range of densities across the freezing line.File in questo prodotto:
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